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Symmetry and Topology Determine the MoV–CN–MnII Exchange Interactions in High-Spin Molecules.
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- Angewandte Chemie International Edition, 2005, v. 44, n. 18, p. 2711, doi. 10.1002/anie.200500129
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Ultra-rapid Synthesis of 15O-Labeled 2-Deoxy-D-glucose for Positron Emission Tomography (PET)This work was supported by a Grant-in-Aid for the 21st century COE Program for Frontiers in Fundamental Chemistry from the Ministry of Education, Culture, Sports, Science, and Technology of Japan (to E.N.), and by a postdoctoral research fellowship for SPD from the Japan Society for the Promotion of Science (to H.Y.). We thank Dr. Akihiro Noda for assistance with PPIS imaging and Dr. Masahiro Yamanaka and Dr. Cecile Savarin for their important previous contributions.
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- Angewandte Chemie International Edition, 2005, v. 44, n. 18, p. 2708, doi. 10.1002/anie.200500044
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Preview: Angew. Chem. Int. Ed. 18/2005.
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- Angewandte Chemie International Edition, 2005, v. 44, n. 18, p. 2813, doi. 10.1002/anie.200590062
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Graphical Abstract: Angew. Chem. Int. Ed. 18/2005.
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- Angewandte Chemie International Edition, 2005, v. 44, n. 18, p. 2616, doi. 10.1002/anie.200590061
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Cover Picture: Branching Out of Single-Molecule Fluorescence Spectroscopy: Challenges for Chemistry and Influence on Biology (Angew. Chem. Int. Ed. 18/2005).
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- Angewandte Chemie International Edition, 2005, v. 44, n. 18, p. 2613, doi. 10.1002/anie.200590060
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Destinctions for Materials Scientists Rao, Whitesides, and Langer.
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- Angewandte Chemie International Edition, 2005, v. 44, n. 18, p. 2628, doi. 10.1002/anie.200501179
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Total Synthesis of (−)-Laulimalide: Pd-Catalyzed Stereospecific Ring Construction of the Substituted 3,6-Dihydro[2H]pyran UnitsThis research was supported (in part) by the 21st COE Program from the Ministry of Education, Science and Culture of Japan. We appreciate Dr. B. M. Gallagher, Jr. (Eisai Research Institute) for providing a copy of NMR charts for the seco acid 20 and (−)-laulimalide 1.
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- Angewandte Chemie International Edition, 2005, v. 44, n. 18, p. 2756, doi. 10.1002/anie.200500029
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New Developments in the Asymmetric Stetter ReactionThe author thanks the Fonds der Chemischen Industrie for a Liebig fellowship.
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- Angewandte Chemie International Edition, 2005, v. 44, n. 18, p. 2632, doi. 10.1002/anie.200500761
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Genetically Selected Cyclic-Peptide Inhibitors of AICAR Transformylase HomodimerizationWe thank A. R. Horswill, T. A. Naumann, S. W. Nelson, S. N. Savinov, and M. E. Webb for helpful discussions. This work was funded by National Institutes of Health grant GM24129-28. AICAR=aminoimidazole-4-carboxamide ribonucleotide.
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- Angewandte Chemie International Edition, 2005, v. 44, n. 18, p. 2760, doi. 10.1002/anie.200500417
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Copper-Catalyzed Enantioselective Conjugate Addition of Grignard Reagents to α,β-Unsaturated EstersFinancial support from the Dutch Ministry of Economic Affairs under the EET Scheme (grant nos. EETK97107 and EETK99104) and the Sixth Framework Programme of the European Community (Marie Curie Intra-European Fellowship to F.L.; contract no: MEIF-CT-2004-009767) is gratefully acknowledged. We thank T. D. Tiemersma-Wegman for technical support (GC and HPLC) and Dr. W. R. Browne for valuable discussions. We are grateful to Dr. H.-U. Blaser (Solvias, Basel) for a generous gift of josiphos ligands.
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- Angewandte Chemie International Edition, 2005, v. 44, n. 18, p. 2752
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Total Synthesis of Antascomicin BThe authors would like to thank Novartis for the Novartis Research Fellowship (to S.V.L.), Trinity College, Cambridge for a Junior Research Fellowship (to D.E.A.B.), Pembroke College, Cambridge and the Royal Society for fellowships (to M.D.S.), the EPSRC (to C.M.G.-J., M.R.L., C.M., and D.E.A.B.), Tanabe Seiyaku Co., Ltd. for a postdoctoral fellowship (to K.Y.), and the Japanese Society for the Promotion of Sciences (to R.A.). The authors would also like to acknowledge the contribution of Prof. Hidenori Watanabe (University of Tokyo; Cambridge 1998–2000) whose studies on a related system were invaluable in the development of the macrocyclization method described herein.
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- Angewandte Chemie International Edition, 2005, v. 44, n. 18, p. 2732, doi. 10.1002/anie.200500174
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Effect of the Metal-Assisted Assembling Mode on the Redox States of Hexaazatriphenylene HexacarbonitrileWe would like to thank Prof. Dr. Takashi Kawamura and Dr. Ryo Kitaura for their help with the DFT calculations. This work was supported by a Grant-In-Aid for Science Research from the Ministry of Education, Culture, Sports, Science and Technology, Japan. S.F. is grateful to the JSPS Research Fellowships for Young Scientists.
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- Angewandte Chemie International Edition, 2005, v. 44, n. 18, p. 2700, doi. 10.1002/anie.200462962
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Gold Catalysis: Proof of Arene Oxides as Intermediates in the Phenol SynthesisThis work was supported by the Fonds der Chemischen Industrie, in particular through a Chemiefonds-Doktoranden-Stipendium to J.P.W., and by the AURICAT EU-RTN (HPRN-CT-2002-00174).
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- Angewandte Chemie International Edition, 2005, v. 44, n. 18, p. 2798, doi. 10.1002/anie.200462672
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Monodisperse Magnetic Single-Crystal Ferrite MicrospheresThis work was supported by the NSFC (90 406 003, 20 401 010, 50 372 030, 20 025 102, 20 131 030), the Foundation for the Author of National Excellent Doctoral Dissertation of the P.R. China, and the state key project of fundamental research for nanomaterials and nanostructures (2003CB716901).
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- Angewandte Chemie International Edition, 2005, v. 44, n. 18, p. 2782, doi. 10.1002/anie.200462551
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Molecular Recognition by Glycoside Pseudo Base Pairs and Triples in an Apramycin–RNA ComplexThis work was supported by the National Institutes of Health (Grant no. AI51104 to T.H.).
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- Angewandte Chemie International Edition, 2005, v. 44, n. 18, p. 2694, doi. 10.1002/anie.200500028
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Strong Means Slow: Dynamic Contributions to the Bulk Mechanical Properties of Supramolecular NetworksThis work was supported by the Petroleum Research Fund of the American Chemical Society and Duke University. Partial support was provided by the North Carolina Biotechnology Center and Research Corp. D.M.L. is an NSF IGERT Fellow (DGE-0221632). S.L.C. gratefully acknowledges a DuPont Young Professor Award and a Camille and Henry Dreyfus New Faculty Award. We thank S. Zauscher for access to his rheometer, T. Ribiero for assistance with the dynamic NMR spectroscopy experiments, and T. Al-Tel for helpful conversations.
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- Angewandte Chemie International Edition, 2005, v. 44, n. 18, p. 2746, doi. 10.1002/anie.200500026
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Synthetic Multivalent Molecules. Concepts and Biomedical Applications. By Seok-Ki Choi.
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- Angewandte Chemie International Edition, 2005, v. 44, n. 18, p. 2629, doi. 10.1002/anie.200485266
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Redox-Induced Transformation from an Extended to a π-Stacked Conformer in Acyclic Bis(catecholacetal)s of AcetylacetoneWe thank the National Science Foundation (Career Award) and the donors of the Petroleum Research Fund (AC12345), administered by the American Chemical Society, for financial support.
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- Angewandte Chemie International Edition, 2005, v. 44, n. 18, p. 2771, doi. 10.1002/anie.200463103
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Molecular Basis of Perhydrolase Activity in Serine HydrolasesWe thank the Swedish Foundation for International Cooperation in Research and Higher Education (STINT) and the University of Minnesota for financial support, the Minnesota Supercomputing Institute for computer modeling resources, C. Savile for advice and discussions, and M. Smith and J. Gosse for initial work.
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- Angewandte Chemie International Edition, 2005, v. 44, n. 18, p. 2742, doi. 10.1002/anie.200463006
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Uniform, Axial-Orientation Alignment of One-Dimensional Single-Crystal Silicon Nanostructure ArraysThis work was supported by the National Natural Science Foundation, National 973 Project of the People's Republic of China, and 985 Project of Tsinghua University.
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- Angewandte Chemie International Edition, 2005, v. 44, n. 18, p. 2737, doi. 10.1002/anie.200462995
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Preventing Crystallization of Phospholipids in Monolayers: A New Approach to Lung-Surfactant TherapyWe thank Alliance Pharmaceutical Corporation (San Diego, CA, USA) for the gift of perfluorooctyl bromide.
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- Angewandte Chemie International Edition, 2005, v. 44, n. 18, p. 2749, doi. 10.1002/anie.200462978
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Asymmetric Amplification Using Chiral Cocrystals Formed from Achiral Organic Molecules by Asymmetric AutocatalysisThis work was supported by a Grant-in-Aid for Scientific Research from The Ministry of Education, Culture, Sports, Science, and Technology (MEXT).
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- Angewandte Chemie International Edition, 2005, v. 44, n. 18, p. 2774, doi. 10.1002/anie.200462963
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Beyond Oil and Gas: The Methanol EconomyAn identically titled monograph that discusses various aspects of the methanol economy is being published by Wiley-VCH.
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- Angewandte Chemie International Edition, 2005, v. 44, n. 18, p. 2636, doi. 10.1002/anie.200462121
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From AgCN Chains to a Fivefold Helix and a Fishnet-Shaped Framework StructureWe thank Mrs. Irene Brüdgam for performing the diffraction measurements.
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- Angewandte Chemie International Edition, 2005, v. 44, n. 18, p. 2794, doi. 10.1002/anie.200462793
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DNA Detection through Signal Amplification by Using NADH:Flavin Oxidoreductase and Oligonucleotide–Flavin Conjugates as CofactorsNADH=nicotinamide adenine dinucleotide, reduced form. This work was supported by the CNRS program “Puces à ADN”.
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- Angewandte Chemie International Edition, 2005, v. 44, n. 18, p. 2764, doi. 10.1002/anie.200461145
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Reversible Binding of Dioxygen by a Non-Transition-Metal ComplexThis work was supported by the Russian Foundation for Basic Research (grant 04-03-32409) and the Russian President Grant supporting scientific schools (grant no. 1649.2003.3).
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- Angewandte Chemie International Edition, 2005, v. 44, n. 18, p. 2767, doi. 10.1002/anie.200462503
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Supercritical Water as a Solvent.
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- Angewandte Chemie International Edition, 2005, v. 44, n. 18, p. 2672
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An Exceptionally Selective Lead(II)-Regulatory Protein from Ralstonia Metallidurans: Development of a Fluorescent Lead(II) ProbeThis work was supported by the University of Chicago and a Searle Scholar award to C.H. P.C. is supported by the Burroughs Wellcome Fund Cross-Disciplinary Training Program (grant no.: 1001774C). The work by B.G., S.T., and D.v.d.L. was supported by Laboratory Directed Research and Development funds at the Brookhaven National Laboratory under contract with the US Department of Energy. We thank Dr. J. Piccirilli for the use of the DNA synthesizer, Dr. N.-S. Li, E. M. Duguid, and Y. Mishina for assistance with DNA synthesis, and the Biophysics Core Facility at the University of Chicago, and Dr. M. A. Yousef for help with fluorescence and isothermal titration calorimetry measurements.
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- Angewandte Chemie International Edition, 2005, v. 44, n. 18, p. 2715, doi. 10.1002/anie.200462443
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Quantitative Dynamic Interconversion between AgI-Mediated Capsule and Cage Complexes Accompanying Guest Encapsulation/ReleaseThis work was supported by a Grant-in-Aid for The 21 st Century COE Program for Frontiers in Fundamental Chemistry and by Grants-in-Aid for Scientific Research (S) to M.S. (No. 16 105 001) and for Scientific Research on Priority Areas, “Dynamic Complexes” to S.H. (No. 420/16033215) from the Ministry of Education, Culture, Sports, Science, and Technology of Japan.
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- Angewandte Chemie International Edition, 2005, v. 44, n. 18, p. 2727, doi. 10.1002/anie.200462394
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Active Sites on Oxide Surfaces: ZnO-Catalyzed Synthesis of Methanol from CO and H2This research was supported by the German Science Foundation within the framework of the Collaborative Research Center 558 “Metal–Substrate Interactions in Heterogeneous Catalysis”.
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- Angewandte Chemie International Edition, 2005, v. 44, n. 18, p. 2790, doi. 10.1002/anie.200462374
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Discotic Liquid Crystals with an Inverted StructureFinancial Support by the Deutsche Forschungsgemeinschaft is gratefully acknowledged.
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- Angewandte Chemie International Edition, 2005, v. 44, n. 18, p. 2801, doi. 10.1002/anie.200462319
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Terphenyl-Based Helical Mimetics That Disrupt the p53/HDM2 InteractionWe thank the National Institutes of Health for support of this work (GM35208 and GM69850). The HDM2 pQE40 construct was kindly provided by Dr. Christian Klein (Hoffmann-La Roche, Inc.).
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- Angewandte Chemie International Edition, 2005, v. 44, n. 18, p. 2704, doi. 10.1002/anie.200462316
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Wound Closure in the Invasive Green Alga Caulerpa taxifolia by Enzymatic Activation of a Protein Cross-LinkerWe thank the Deutsche Forschungsgemeinschaft for funding. Prof. W. Boland is gratefully acknowledged for support, Dr. B. Schneider for help with NMR spectroscopic measurements, and A. Perner for HRMS measurements.
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- Angewandte Chemie International Edition, 2005, v. 44, n. 18, p. 2806, doi. 10.1002/anie.200462276
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Chasing a Phantom by Total Synthesis: The Butylcycloheptylprodigiosin CaseGenerous financial support from the Deutsche Forschungsgemeinschaft (Leibniz award program), the Fonds der Chemischen Industrie, and the Merck Research Council is gratefully acknowledged. We thank Dr. R. Mynott and C. Wirtz for their invaluable help with numerous NMR analyses and Prof. H. Floss for providing a copy of the 1H NMR spectrum of his “pink pigment” for comparison.
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- Angewandte Chemie International Edition, 2005, v. 44, n. 18, p. 2777, doi. 10.1002/anie.200462215
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Direct Detection of Inter-residue Hydrogen Bonds in Polysaccharides by Single-Molecule Force SpectroscopyThis work was supported by a grant from the National Science Foundation and by Duke University funds to P.E.M. We thank Prof. Yasuhiro Takahashi of Osaka University, Japan for a sample of amylose triacetate.
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- Angewandte Chemie International Edition, 2005, v. 44, n. 18, p. 2723, doi. 10.1002/anie.200462067
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Proton Sandwiches: Nonclassical Carbocations with Tetracoordinate ProtonsWe gratefully acknowledge the University of California, Davis, and the National Computational Science Alliance for support of this research, and we thank P. von R. Schleyer for helpful comments.
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- Angewandte Chemie International Edition, 2005, v. 44, n. 18, p. 2719, doi. 10.1002/anie.200461915
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Scaling the Alignment of Small Organic Molecules in Substituted Polyglutamates by Variable-Angle Sample SpinningThis work was supported by the Fonds der Chemischen Industrie. I thank Prof. Dr. S. Berger, Dr. P. Lesot, Dr. M. Zweckstetter, and Prof. Dr. D. Freude for their help.
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- Angewandte Chemie International Edition, 2005, v. 44, n. 18, p. 2787, doi. 10.1002/anie.200461532
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Branching Out of Single-Molecule Fluorescence Spectroscopy: Challenges for Chemistry and Influence on Biology.
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- Angewandte Chemie International Edition, 2005, v. 44, n. 18, p. 2642, doi. 10.1002/anie.200300647
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