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- Title
Impact of mixing state and hygroscopicity on CCN activity of biomass burning aerosol in Amazonia.
- Authors
Gácita, Madeleine Sánchez; Longo, Karla M.; Freire, Julliana L. M.; Freitas, Saulo R.; Martin, Scot T.
- Abstract
Smoke aerosols prevail throughout Amazonia because of widespread biomass burning during the dry season. External mixing, low variability in the particle size distribution and low particle hygroscopicity are typical. There can be profound effects on cloud properties. This study uses an adiabatic cloud model to simulate the activation of smoke particles as cloud condensation nuclei (CCN) and to assess the relative importance of variability in hygroscopicity, mixing state, and activation kinetics for the activated fraction and maximum supersaturation. The analysis shows that use of medium values of hygroscopicity representative of smoke aerosols for other biomass burning regions on Earth can lead to significant errors, compared to the use of low hygroscopicity reported for Amazonia. Kinetic limitations, which can be significant for medium and high hygroscopicity, did not play a strong role for CCN activation of particles representative of Amazonia smoke aerosols, even when taking into account the large aerosol mass and number concentrations typical of the region. Internal compared to external mixing of particle components of variable hygroscopicity resulted in a significant overestimation of the activated fraction. These findings on uncertainties and sensitivities provide guidance on appropriate simplifications that can be used for modeling of smoke aerosols within general circulation models.
- Subjects
AMAZON River Region; CLOUD condensation nuclei; MIXING; BIOMASS burning; PARTICLE size distribution; ATMOSPHERIC aerosols
- Publication
Atmospheric Chemistry & Physics Discussions, 2016, p1
- ISSN
1680-7367
- Publication type
Article
- DOI
10.5194/acp-2016-248