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- Title
Catalytic Fast Pyrolysis of Biomass into Aromatic Hydrocarbons over Mo-Modified ZSM-5 Catalysts.
- Authors
Sun, Laizhi; Wang, Zhibin; Chen, Lei; Yang, Shuangxia; Xie, Xinping; Gao, Mingjie; Zhao, Baofeng; Si, Hongyu; Li, Jian; Hua, Dongliang
- Abstract
Mo-modified ZSM-5 catalysts were prepared and used to produce aromatic hydrocarbons during catalytic fast pyrolysis (CFP) of biomass. The composition and distribution of aromatics were investigated on pyrolysis–gas chromatography/mass spectrometry (Py-GC/MS). The reaction factors, such as the Mo content, the reaction temperature and the catalyst/biomass mass ratio, were also optimized. It was found that the 10Mo/ZSM-5 catalyst displayed the best activity in improving the production of monocyclic aromatic hydrocarbons (MAHs) and decreasing the yield of polycyclic aromatic hydrocarbons (PAHs) at 600 °C and with a catalyst/biomass ratio of 10. Furthermore, according to catalyst characterization and the experiment results, the aromatics formation mechanism over Mo/ZSM-5 catalysts was also summarized and proposed.
- Subjects
AROMATIC compounds; BIOMASS; POLYCYCLIC aromatic hydrocarbons; CATALYSTS; PYROLYSIS gas chromatography; MOLYBDENUM disulfide
- Publication
Catalysts (2073-4344), 2020, Vol 10, Issue 9, p1051
- ISSN
2073-4344
- Publication type
Article
- DOI
10.3390/catal10091051