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- Title
Methane emissions from China: a high-resolution inversion of TROPOMI satellite observations.
- Authors
Zichong Chen; Jacob, Daniel J.; Nesser, Hannah; Sulprizio, Melissa P.; Lorente, Alba; Varon, Daniel J.; Xiao Lu; Lu Shen; Zhen Qu; Elise Penn; Xueying Yu
- Abstract
We quantify methane emissions in China and the contributions from different sectors by inverse analysis of 2019 TROPOMI satellite observations of atmospheric methane. The inversion uses as prior estimate the national sector-resolved anthropogenic emission inventory reported by the Chinese government to the United Nations Framework Convention on Climate Change (UNFCCC) and thus serves as a direct evaluation of that inventory. Emissions are optimized with a Gaussian mixture model (GMM) at up to 0.25o×0.3125o resolution. The optimization is done analytically assuming lognormally distributed errors on prior emissions. Errors and information content on the optimal estimates are obtained directly from the analytical solution and also through a 36-member inversion ensemble. Our optimal estimate for total anthropogenic emissions in China is 65.0 (57.7-68.4) Tg a-1, where parentheses indicate uncertainty range. Contributions from individual sectors include 16.6 (15.6-17.6) Tg a-1 for coal, 2.3 (1.8-2.5) for oil, 0.29 (0.23-0.32) for gas, 17.8 (15.1-21.0) for livestock, 9.3 (8.2-9.9) for waste, 11.9 (10.7-12.7) for rice paddies, and 6.7 (5.8-7.1) for other sources. Our estimate is 21% higher than the Chinese inventory reported to the UNFCCC (53.6 Tg a-1), reflecting upward corrections to emissions from oil (+147%), gas (+61%), livestock (+37%), waste (+41%), and rice paddies (+34%), but downward correction for coal (-15%). It is also higher than previous inverse studies (43-62 Tg a-1) that used the much sparser GOSAT satellite observations and were conducted at coarser resolution. We are in particular better able to separate coal and rice emissions. Our higher livestock emissions are attributed largely to northern China where GOSAT has little sensitivity. Our higher waste emissions reflect at least in part a rapid growth in wastewater treatment in China. Underestimate of oil emissions in the UNFCCC report appears to reflect unaccounted super-emitting facilities. Gas emissions in China are mostly from distribution, in part because of low emission factors from production and in part because 42% of the gas is imported. Our estimate of emissions per unit of domestic gas production indicates a low life-cycle loss rate of 1.7 (1.3-1.9) %, which would imply net climate benefits from the current coal-to-gas energy transition in China. However, this small loss rate is somewhat misleading considering China's high gas imports, including from Turkmenistan where emission per unit of gas production is very high.
- Subjects
CHINA; GAUSSIAN mixture models; EMISSION inventories; ATMOSPHERIC methane; PADDY fields; METHANE; WASTEWATER treatment
- Publication
Atmospheric Chemistry & Physics Discussions, 2022, p1
- ISSN
1680-7367
- Publication type
Article
- DOI
10.5194/acp-2022-303