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- Title
A Ratiometric Fluorescent Probe Dye-Functionalized MOFs Integrated with Logic Gate Operation for Efficient Detection of Acetaldehyde.
- Authors
Wenwei Li; Min Liu; Yourong Zhao; Yangchun Fan; Yuting Li; Hongmei Gao; Hongda Li; Daojiang Gao; Zhanglei Ning
- Abstract
Volatile organic compounds (VOCs) are a class of hazardous gases that are widely present in the atmosphere and cause great harm to human health. In this paper, a ratiometric fluorescent probe (Dye@Eu-MOFs) based on a dye-functionalized metal–organic framework was designed to detect VOCs, which showed high sensitivity and specificity for acetaldehyde solution and vapor. A linear correlation between the integrated fluorescence intensity (I510/I616) and the concentration of acetaldehyde was investigated, enabling a quantitative analysis of acetaldehyde in the ranges of 1 × 10−4~10−5 µL/mL, with a low detection limit of 8.12 × 10−4 mg/L. The selective recognition of acetaldehyde could be clearly distinguished by the naked eye under the excitation of UV light. The potential sensing mechanism was also discussed. Significantly, a molecular logic gate was constructed based on the whole system, and finally, a molecular logic network system for acetaldehyde detection connecting basic and integrated logic operations was realized. This strategy provided an effective guiding method for constructing a molecular-level logic gate for acetaldehyde detection on a simple platform.
- Publication
Molecules, 2024, Vol 29, Issue 13, p1
- ISSN
1420-3049
- Publication type
Article
- DOI
10.3390/molecules29132970