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- Title
Dehydrogenative Aromatization and Sulfonylation of Pyrrolidines: Orthogonal Reactivity in Photoredox Catalysis.
- Authors
Muralirajan, Krishnamoorthy; Kancherla, Rajesh; Rueping, Magnus
- Abstract
Oxidative dehydrogenative aromatization and selective sulfonylation reactions of N‐heterocycles under visible‐light photoredox catalysis were established. The mild reaction conditions make this approach an appealing and versatile strategy to functionalize/oxidize pyrrolidines whereby arylsulfonyl chlorides were identified to be both catalyst regeneration and sulfonylation reagents.
- Subjects
DEHYDROGENATION; AROMATIZATION catalysts; REACTIVITY (Chemistry); PYRROLIDINE; OXIDATION-reduction reaction; SULFONYL chlorides
- Publication
Angewandte Chemie, 2018, Vol 130, Issue 45, p15003
- ISSN
0044-8249
- Publication type
Article
- DOI
10.1002/ange.201808427