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- Title
UV to NIR Broadband Flexible Photodetector Based on Solution‐Processed MoS<sub>2</sub>/PDPP3T Inorganic–Organic Hybrid Heterostructures.
- Authors
Tang, Daxiu; Du, Zhenyu; Xie, Ying; Zhao, Feiyu; Yang, Xiangdong; Gu, Chenjie; Shen, Xiang
- Abstract
Molybdenum disulfide (MoS2) is a 2D material with excellent electrical and optical properties, and developing a universal technology for the preparation of high‐performance MoS2‐based photodetector is extremely desirable. Here, a UV to NIR broadband flexible photodetector based on MoS2/(PDPP3T) inorganic–organic hybrid heterostructures is reported. In the experiment, high crystalline 2H‐phase few‐layer MoS2 nanoflakes are first prepared by optimized electrochemical intercalation of tetraheptylammonium cation (THA+) and ultrasound‐assisted exfoliation strategy. Thereafter, a narrow bandgap organic semiconductor PDPP3T is introduced to construct the MoS2/Poly(diketopyrrolopyrrolothiophrn) (PDPP3T) heterojunction. Experimental results reveal that the photodetector can have broadband photo response from 380 to 980 nm. Meanwhile, excellent responsivities and detectivity of 12.4 mA W−1, 2.2 × 1010 Jones at 380 nm and 0.1 mA W−1 and 5 × 108 Jones at 980 nm are achieved, which are ≈10 (UV band)/100 (NIR band) times high than that obtained on the pure MoS2‐based detector. Moreover, the flexibility of the device is investigated by conformal covering the device on a curved surface (R = 5 and 2.5 mm), it shows that the photo response remains almost the same as that measured on the planar substrate, indicating the possible application in the wearable electronics.
- Subjects
PHOTODETECTORS; HETEROSTRUCTURES; ORGANIC semiconductors; MOLYBDENUM disulfide; CURVED surfaces; NEAR infrared radiation
- Publication
Advanced Materials Interfaces, 2024, Vol 11, Issue 17, p1
- ISSN
2196-7350
- Publication type
Article
- DOI
10.1002/admi.202301065