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- Title
Three-Dimensional Graphene-Magnetic Palladium Nanohybrid: A Highly Efficient and Reusable Catalyst for Promoting Organic Reactions.
- Authors
Tanhaei, Mahboobeh; Mahjoub, Alireza; Nejat, Razieh
- Abstract
Abstract: In this work, graphene aerogel (GA) decorated with Fe3O4@SiO2@Pd nanoparticles (GA-FSNP@Pd) as a novel three-dimensional graphene-magnetic palladium nanohybrid catalyst. This catalyst showed high catalytic activity for the Suzuki and Heck cross-coupling reactions. This noteworthy catalyst activity can be due to the high dispersion of FSNP@Pd nanoparticles on GA. The nanohybrid exhibits an interconnected mesoporous framework of graphene sheets with uniform dispersion of FSNP@Pd nanoparticles. Interestingly, the catalyst could be recovered in a facile manner from the reaction mixture and recycled ten times without appreciable loss of activity. High yield, low reaction time, magnetic separation and non-toxicity of the nanohybrid catalyst are the main merits of this protocol.Graphical Abstract: <graphic></graphic>
- Subjects
PALLADIUM catalysts; CATALYTIC activity; GRAPHENE; COUPLING reactions (Chemistry); AEROGELS; MESOPOROUS materials
- Publication
Catalysis Letters, 2018, Vol 148, Issue 6, p1549
- ISSN
1011-372X
- Publication type
Article
- DOI
10.1007/s10562-018-2347-y