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- Title
3D Printed Design‐Assisted Multilayered Graphene Oxide‐Modified Polymer Glucose Sensor.
- Authors
Das, Chirantan; Das, Subham; Chugh, Vibhas; Bhattacharjee, Mitradip
- Abstract
This work investigates the capabilities of a platform for nonenzymatic glucose sensing employing a novel 3D printed three‐electrode mask‐embedded design. A reservoir‐on‐mask has been fabricated for smart sample insertion to avoid spillage. Working and counter silver electrodes are modified with three different material combinations such as graphene oxide (GO), poly(3,4‐ethylenedioxythiophene):poly(styrenesulfonate) (PEDOT:PSS), and GO + PEDOT:PSS, and their performance comparison is demonstrated. It is observed that the GO + PEDOT:PSS modification shows 94.57 and 71.01% higher sensitivity than GO and PEDOT:PSS, respectively, including a higher linearity compared to its counterparts. Glucose concentrations ranging from 50 to 300 mg dL−1 are detected by employing cyclic voltammetry and electrical impedance spectroscopic technique. Herein, a significantly high sensitivity of 18.8 μAmM−1 cm−2 and low limit of detection ≈ 0.4 mM has been achieved for the proposed sensor. The 3D printed mask structure provides 75% higher sample retention ability, greater reliability in terms of sample placement in the sensor and improved test performances. The proposed sensor can provide a stable and large‐scale deployable solution to future biosensing platforms.
- Subjects
ELECTRIC impedance; SILVERWORK; GRAPHENE; SENSOR placement; CYCLIC voltammetry; CONDUCTING polymers
- Publication
Advanced Engineering Materials, 2024, Vol 26, Issue 1, p1
- ISSN
1438-1656
- Publication type
Article
- DOI
10.1002/adem.202301067