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- Title
Narrowing the Gap between Theoretical and Practical Capacities in Li-Ion Layered Oxide Cathode Materials.
- Authors
Radin, Maxwell D.; Hy, Sunny; Sina, Mahsa; Fang, Chengcheng; Liu, Haodong; Vinckeviciute, Julija; Zhang, Minghao; Whittingham, M. Stanley; Meng, Y. Shirley; Van der Ven, Anton
- Abstract
Although layered lithium oxides have become the cathode of choice for state-of-the-art Li-ion batteries, substantial gaps remain between the practical and theoretical energy densities. With the aim of supporting efforts to close this gap, this work reviews the fundamental operating mechanisms and challenges of Li intercalation in layered oxides, contrasts how these challenges play out differently for different materials (with emphasis on Ni-Co-Al (NCA) and Ni-Mn-Co (NMC) alloys), and summarizes the extensive corpus of modifications and extensions to the layered lithium oxides. Particular emphasis is given to the fundamental mechanisms behind the operation and degradation of layered intercalation electrode materials as well as novel modifications and extensions, including Na-ion and cation-disordered materials.
- Subjects
LITHIUM-ion batteries; CATHODES; ENERGY density; CLATHRATE compounds; LITHIUM tantalate
- Publication
Advanced Energy Materials, 2017, Vol 7, Issue 20, pn/a
- ISSN
1614-6832
- Publication type
Article
- DOI
10.1002/aenm.201602888