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- Title
Branching of the intermediate N<sub>2</sub>O decomposition in a steady-state NO + CO + O<sub>2</sub> reaction on Pd(110); an angle-resolved desorption study.
- Authors
Ma, Y.; Rzeznicka, I.; Matsushima, T.
- Abstract
The branching of the intermediate N2O decomposition vs. the desorption was studied in a steady-state NO + CO + O2 reaction on Pd(110). Three surface-nitrogen removal processes, i.e., N2O(a) ? N2(g) + O(a), N2O(a) ? N2O(g) and 2N(a) ? N2(g), are operative. Only about 20% of N2O(a) was desorbed without decomposition for a (NO:CO = 1:1) mixture. The fraction increased steeply with increasing surface oxygen.
- Subjects
ALUMINUM silicates; CATALYSIS; CHEMICAL reactions; CHEMICAL processes; PHYSICAL &; theoretical chemistry
- Publication
Catalysis Letters, 2005, Vol 101, Issue 1/2, p109
- ISSN
1011-372X
- Publication type
Article
- DOI
10.1007/s10562-005-3758-0