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- Title
Velocity map imaging VUV angle-resolved photoelectron spectroscopy of isolated silver sulfide nanoparticles.
- Authors
Danilović, Danijela; Božanić, Dušan K.; Garcia, Gustavo A.; Nahon, Laurent; Stamenović, Una; Vodnik, Vesna V.; Djoković, Vladimir
- Abstract
The angle-resolved photoelectron spectroscopy of isolated silver sulfide nanoparticles was carried out by using velocity map imaging technique at the DESIRS beamline of SOLEIL synchrotron facility. The reported spectroscopy results were obtained after interaction of the synchrotron radiation with a polydisperse aerosol produced from aqueous dispersion of silver sulfide particles, approximately 16 nm in diameter. The photoelectron and UV–Vis-NIR absorption spectra were used to estimate the maximum energy of the valance- and the minimum energy of the conduction-band of the nanoparticles. With respect to the vacuum level, the obtained values were found to be 5.5 ± 0.1 eV and 4.5 ± 0.1 eV for the valence band maximum and conduction band minimum, respectively. The dependence of the asymmetry parameter on the electron energy along the silver sulfide valence band showed an onset of inelastic scattering at ~ 1 eV electron kinetic energy.
- Subjects
SILVER sulfide; PHOTOELECTRON spectroscopy; SILVER nanoparticles; SYNCHROTRON radiation; ELECTRON kinetic energy; CONDUCTION bands; INELASTIC scattering; PHOTOELECTRONS
- Publication
Optical & Quantum Electronics, 2022, Vol 54, Issue 9, p1
- ISSN
0306-8919
- Publication type
Article
- DOI
10.1007/s11082-022-03972-6