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- Title
Metal Poly(heptazine imides) as Multifunctional Photocatalysts for Solar Fuel Production.
- Authors
Pelicano, Christian Mark; Antonietti, Markus
- Abstract
Solar‐driven photocatalysis employing particulate semiconductors represents a promising approach for sustainable production of valuable chemical feedstock. Metal poly(heptazine imide) (MPHI), a novel 2D ionic carbon nitride, has been recognized as an emerging photocatalyst with distinctive properties. In this minireview, we first delineate the forefront innovations of MPHI photocatalysts, spanning from synthetic strategies and solving structures to the exploration of novel properties. We place special emphasis on the structural design principles aimed at developing high‐performance MPHI systems toward photocatalytic solar fuel production such as H2 evolution, H2O oxidation, H2O2 production and CO2 reduction. Finally, we discuss crucial insights and challenges in leveraging highly active MPHIs for efficient solar‐to‐chemical energy conversion.
- Subjects
PHOTOCATALYSTS; SUSTAINABILITY; IMIDES; METALS; ENERGY conversion; NITRIDES
- Publication
Angewandte Chemie, 2024, Vol 136, Issue 24, p1
- ISSN
0044-8249
- Publication type
Article
- DOI
10.1002/ange.202406290