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- Title
Interface Regulation via Electric Double Layer for Rechargeable Batteries.
- Authors
Du, Haiying; Song, Keming; Yang, Mingrui; Huang, Peng; Chen, Weihua
- Abstract
Interphases, especially the electrochemically formed solid electrolyte interphase (SEI), are significantly important for cycling stability, reaction kinetics and safety of rechargeable batteries. The structure and composition of the electric double layer (EDL) greatly affect the formation of the SEI and the performance of electrodes. However, as far as we know, there is no review discussing the theme specifically. Herein, the recent substantial progress for EDL and its impact on the formation of SEI in rechargeable batteries are reviewed and discussed. Firstly, the specific adsorption of electrolyte components on electrodes' surface and the ionic solvation structure are introduced. Furthermore, various methods for controlling EDL in different electrode systems are described. Finally, the potential future advancements of the SEI through the manipulation of EDL are discussed, aiming to enhance the electrochemical performance of rechargeable batteries.
- Subjects
ELECTRIC double layer; STORAGE batteries; ELECTRODE performance; SOLID electrolytes; IONIC structure; ELECTRIC batteries
- Publication
ChemSusChem, 2023, Vol 16, Issue 24, p1
- ISSN
1864-5631
- Publication type
Article
- DOI
10.1002/cssc.202300708